Universal and state-resolved imaging of chemical dynamics

David Townsend; Wen Li; Suk Kyoung Lee; Richard L Gross; Arthur G Suits

doi:10.1021/jp0526086

Universal and state-resolved imaging of chemical dynamics

David Townsend
, Wen Li
, Suk Kyoung Lee
, Richard L Gross
, Arthur G Suits

Research output: Contribution to journal › Article › peer-review

51 Citations (Scopus)

Abstract

We showcase the use of high-resolution ion imaging with complementary state-resolved and "universal" vacuum ultraviolet probes to address a broad range of fundamental problems in chemical reaction dynamics. Examples from our recent work include applications in state-correlated unimolecular reactions, ion pair dissociation dynamics and spectroscopy, crossed-beam reactive scattering, and atomic angular momentum polarization in photodissociation. These studies are all directed to achieving a detailed understanding of atomic and molecular interactions, with particular emphasis on reaction mechanisms outside the scope of transition state theory; on spectroscopy and dynamics of highly excited, transient species; on nonadiabatic reaction mechanisms; and on chemical dynamics in polyatornic systems.

Original language	English
Pages (from-to)	8661-8674
Number of pages	14
Journal	The Journal of Physical Chemistry A
Volume	109
Issue number	39
DOIs	https://doi.org/10.1021/jp0526086
Publication status	Published - 6 Oct 2005

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AU - Suits, Arthur G

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AB - We showcase the use of high-resolution ion imaging with complementary state-resolved and "universal" vacuum ultraviolet probes to address a broad range of fundamental problems in chemical reaction dynamics. Examples from our recent work include applications in state-correlated unimolecular reactions, ion pair dissociation dynamics and spectroscopy, crossed-beam reactive scattering, and atomic angular momentum polarization in photodissociation. These studies are all directed to achieving a detailed understanding of atomic and molecular interactions, with particular emphasis on reaction mechanisms outside the scope of transition state theory; on spectroscopy and dynamics of highly excited, transient species; on nonadiabatic reaction mechanisms; and on chemical dynamics in polyatornic systems.

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JO - The Journal of Physical Chemistry A

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Universal and state-resolved imaging of chemical dynamics

Abstract

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