@article{225133168af84e92a8ac34f6fc178336,
title = "Towards quantifying subsurface methane emissions from energy wells with integrity failure",
abstract = "The expansion of petroleum resource development has led to growing concern regarding greenhouse gas emissions from fugitive gas migration, which occurs at some wells due to well integrity failure. In this study, we quantify methane surface expression and emissions resulting from gas migration using a number of complementary techniques, and thereby evaluate surface expression processes as well as the strengths and limitations of the monitoring techniques. Methane emissions were found to be highly localized and variable over time. Injected gas reached the surface via preferential pathways through the soils and also along an installed groundwater monitoring well. Cumulative emissions were estimated from flux chamber measurements to be 3.8–6.5% of the injected gas; whereas eddy covariance (EC) data inferred approximately 26% of the injected gas was released to the atmosphere. Together these methods provide enhanced interpretation of surface expression at the site, advance our understanding on fugitive gas migration from integrity compromised energy wells and provide insights to improve monitoring and detection strategies with a view to reducing future greenhouse gas emissions. Moreover that, up to 75% of fugitive gas released at the site remained in the subsurface, shows that capillary barriers will mitigate greenhouse gas emissions from leaky wells; however, may infer greater potential for impacts on groundwater resources, if present.",
keywords = "Dynamic closed chamber, Eddy covariance, Emissions, Gas migration, Methane, Natural gas, Well integrity failure",
author = "Soares, {Julia V.} and Chitra Chopra and {Van De Ven}, {Cole J. C.} and Cahill, {Aaron G.} and Beckie, {Roger D.} and Black, {T. Andrew} and Bethany Ladd and Mayer, {K. Ulrich}",
note = "Funding Information: We acknowledge this research was conducted in treaty lands of the Treaty 8 First Nations. We would like to thank Dr. and Mrs. Weder of Ventor Ranch for allowing access to the land where the experiment was conducted. This research has been financially supported by Natural Resources Canada (CEI-MET-196B), Geoscience BC (2016-043) and the British Columbia Oil and Gas Research Innovation Society. Funding for equipment for chamber-based soil gas efflux measurements was provided through a Natural Science and Engineering Research Council (NSERC) Research Tools and Instrument (RTI) Grant, a Canada Foundation for Innovation-Leaders of Opportunity Fund (CFI-LOF) grant with matching funding from the British Columbia Knowledge Development Fund (BCKDF), and the BC Oil and Gas Commission. Funding Information: We acknowledge this research was conducted in treaty lands of the Treaty 8 First Nations. We would like to thank Dr. and Mrs. Weder of Ventor Ranch for allowing access to the land where the experiment was conducted. This research has been financially supported by Natural Resources Canada ( CEI-MET-196B ), Geoscience BC (2016-043) and the British Columbia Oil and Gas Research Innovation Society. Funding for equipment for chamber-based soil gas efflux measurements was provided through a Natural Science and Engineering Research Council (NSERC) Research Tools and Instrument (RTI) Grant, a Canada Foundation for Innovation-Leaders of Opportunity Fund (CFI-LOF) grant with matching funding from the British Columbia Knowledge Development Fund (BCKDF) , and the BC Oil and Gas Commission. Publisher Copyright: {\textcopyright} 2021 Turkish National Committee for Air Pollution Research and Control",
year = "2021",
month = dec,
doi = "10.1016/j.apr.2021.101223",
language = "English",
volume = "12",
journal = "Atmospheric Pollution Research",
issn = "1309-1042",
publisher = "Elsevier B.V.",
number = "12",
}