Robust Isolated Attosecond Pulse Generation with Self-Compressed Subcycle Drivers from Hollow Capillary Fibers

Marina Fernández Galán, Javier Serrano, Enrique Conejero Jarque, Rocío Borrego-Varillas, Matteo Lucchini, Maurizio Reduzzi, Mauro Nisoli, Christian Brahms, John C. Travers, Carlos Hernández-García, Julio San Roman

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Abstract

High-order harmonic generation (HHG) arising from the nonperturbative interaction of intense light fields with matter constitutes a well-established tabletop source of coherent extreme-ultraviolet and soft X-ray radiation, which is typically emitted as attosecond pulse trains. However, ultrafast applications increasingly demand isolated attosecond pulses (IAPs), which offer great promise for advancing precision control of electron dynamics. Yet, the direct generation of IAPs typically requires the synthesis of near-single-cycle intense driving fields, which is technologically challenging. In this work, we theoretically demonstrate a novel scheme for the straightforward and compact generation of IAPs from multicycle infrared drivers using hollow capillary fibers (HCFs). Starting from a standard, intense multicycle infrared pulse, a light transient is generated by extreme soliton self-compression in a HCF with decreasing pressure and is subsequently used to drive HHG in a gas target. Owing to the subcycle confinement of the HHG process, high-contrast IAPs are continuously emitted almost independently of the carrier-envelope phase (CEP) of the optimally self-compressed drivers. This results in a CEP-robust scheme which is also stable under macroscopic propagation of the high harmonics in a gas target. Our results open the way to a new generation of integrated all-fiber IAP sources, overcoming the efficiency limitations of usual gating techniques for multicycle drivers.
Original languageEnglish
Pages (from-to)1673-1683
Number of pages11
JournalACS Photonics
Volume11
Issue number4
Early online date18 Mar 2024
DOIs
Publication statusPublished - 17 Apr 2024

Keywords

  • high-order harmonic generation
  • hollow capillary fibers
  • isolated attosecond pulses
  • nonlinear optics
  • soliton self-compression
  • ultrashort laser pulses

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Atomic and Molecular Physics, and Optics
  • Electrical and Electronic Engineering
  • Biotechnology

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