Polarization sensitive spectroscopy of charged quantum dots

E Poem, J. Shemesh, I. Marderfeld, D. Galushko, N Akopian, D Gershoni, Brian D Gerardot, A. Badolato, P M Petroff

Research output: Contribution to journalArticle

66 Citations (Scopus)

Abstract

We present an experimental and theoretical study of the polarized photoluminescence spectrum of single semiconductor quantum dots in various charge states. We compare our high resolution polarization sensitive spectral measurements with a many-carrier model which we developed for this purpose. The model considers both the isotropic and anisotropic exchange interactions between all participating electron-hole pairs. With this addition, we calculate both the energies and polarizations of all optical transitions between collective, quantum dot confined charge-carrier states. We succeed in identifying most of the measured spectral lines. In particular, the lines resulting from singly, doubly, and triply negatively charged excitons and biexcitons. We demonstrate that lines emanating from evenly charged states are linearly polarized. Their polarization direction does not necessarily coincide with the traditional crystallographic direction. It depends on the shells of the single carriers, which participate in the recombination process.

Original languageEnglish
Article number235304
Number of pages12
JournalPhysical Review B: Condensed Matter and Materials Physics
Volume76
Issue number23
DOIs
Publication statusPublished - 15 Dec 2007

Cite this

Poem, E., Shemesh, J., Marderfeld, I., Galushko, D., Akopian, N., Gershoni, D., Gerardot, B. D., Badolato, A., & Petroff, P. M. (2007). Polarization sensitive spectroscopy of charged quantum dots. Physical Review B: Condensed Matter and Materials Physics, 76(23), [235304]. https://doi.org/10.1103/PhysRevB.76.235304