Multi-pass cell driven multi-kHz dispersive wave emission of broadband deep-UV pulses

Laura Silletti; Ammar bin Wahid; Teodora F. Grigorova; Lorenzo Pratolli; Ana Oliveira e Silva; Nans Hermellin; Terry Mullins; Andrea Trabattoni; Christoph M. Heyl; Christian Brahms; Vincent Wanie; John C. Travers; Francesca Calegari

doi:10.1063/5.0268188

Multi-pass cell driven multi-kHz dispersive wave emission of broadband deep-UV pulses

Laura Silletti, Ammar bin Wahid, Teodora F. Grigorova, Lorenzo Pratolli, Ana Oliveira e Silva, Nans Hermellin, Terry Mullins, Andrea Trabattoni, Christoph M. Heyl, Christian Brahms, Vincent Wanie, John C. Travers, Francesca Calegari

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Abstract

In the context of ultrafast spectroscopy, the availability of few-femtosecond UV pulses is key to disclose the role of electron dynamics in photo-activated biochemically relevant processes. Here, we present an optical setup for the generation of UV pulses spectrally tunable between 270 and 350 nm with transform limited durations of 3.0 and 2.9 fs, respectively, and repetition rates up to 50 kHz, using resonant dispersive wave (RDW) emission in an argon-filled hollow-core fiber. The RDW emission is driven by 1030 nm sub-20 fs pulses produced by post-compressing an Yb-based laser with a dispersion-engineered multi-pass cell (MPC). The combination of an MPC with a capillary constitutes a compact source to deliver few-femtosecond UV pulses at high-repetition rates, which is ideal for statistically demanding experiments in molecular physics.

Original language	English
Article number	070801
Journal	APL Photonics
Volume	10
Issue number	7
Early online date	2 Jul 2025
DOIs	https://doi.org/10.1063/5.0268188
Publication status	Published - Jul 2025

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@article{2e73e4c4a83a45b98cc93d7c64645834,

title = "Multi-pass cell driven multi-kHz dispersive wave emission of broadband deep-UV pulses",

abstract = "In the context of ultrafast spectroscopy, the availability of few-femtosecond UV pulses is key to disclose the role of electron dynamics in photo-activated biochemically relevant processes. Here, we present an optical setup for the generation of UV pulses spectrally tunable between 270 and 350 nm with transform limited durations of 3.0 and 2.9 fs, respectively, and repetition rates up to 50 kHz, using resonant dispersive wave (RDW) emission in an argon-filled hollow-core fiber. The RDW emission is driven by 1030 nm sub-20 fs pulses produced by post-compressing an Yb-based laser with a dispersion-engineered multi-pass cell (MPC). The combination of an MPC with a capillary constitutes a compact source to deliver few-femtosecond UV pulses at high-repetition rates, which is ideal for statistically demanding experiments in molecular physics.",

author = "Laura Silletti and Wahid, \{Ammar bin\} and Grigorova, \{Teodora F.\} and Lorenzo Pratolli and \{Oliveira e Silva\}, Ana and Nans Hermellin and Terry Mullins and Andrea Trabattoni and Heyl, \{Christoph M.\} and Christian Brahms and Vincent Wanie and Travers, \{John C.\} and Francesca Calegari",

year = "2025",

month = jul,

doi = "10.1063/5.0268188",

language = "English",

volume = "10",

journal = "APL Photonics",

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publisher = "AIP Publishing",

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T1 - Multi-pass cell driven multi-kHz dispersive wave emission of broadband deep-UV pulses

AU - Silletti, Laura

AU - Wahid, Ammar bin

AU - Grigorova, Teodora F.

AU - Pratolli, Lorenzo

AU - Oliveira e Silva, Ana

AU - Hermellin, Nans

AU - Mullins, Terry

AU - Trabattoni, Andrea

AU - Heyl, Christoph M.

AU - Brahms, Christian

AU - Wanie, Vincent

AU - Travers, John C.

AU - Calegari, Francesca

PY - 2025/7

Y1 - 2025/7

N2 - In the context of ultrafast spectroscopy, the availability of few-femtosecond UV pulses is key to disclose the role of electron dynamics in photo-activated biochemically relevant processes. Here, we present an optical setup for the generation of UV pulses spectrally tunable between 270 and 350 nm with transform limited durations of 3.0 and 2.9 fs, respectively, and repetition rates up to 50 kHz, using resonant dispersive wave (RDW) emission in an argon-filled hollow-core fiber. The RDW emission is driven by 1030 nm sub-20 fs pulses produced by post-compressing an Yb-based laser with a dispersion-engineered multi-pass cell (MPC). The combination of an MPC with a capillary constitutes a compact source to deliver few-femtosecond UV pulses at high-repetition rates, which is ideal for statistically demanding experiments in molecular physics.

AB - In the context of ultrafast spectroscopy, the availability of few-femtosecond UV pulses is key to disclose the role of electron dynamics in photo-activated biochemically relevant processes. Here, we present an optical setup for the generation of UV pulses spectrally tunable between 270 and 350 nm with transform limited durations of 3.0 and 2.9 fs, respectively, and repetition rates up to 50 kHz, using resonant dispersive wave (RDW) emission in an argon-filled hollow-core fiber. The RDW emission is driven by 1030 nm sub-20 fs pulses produced by post-compressing an Yb-based laser with a dispersion-engineered multi-pass cell (MPC). The combination of an MPC with a capillary constitutes a compact source to deliver few-femtosecond UV pulses at high-repetition rates, which is ideal for statistically demanding experiments in molecular physics.

UR - https://www.scopus.com/pages/publications/105009858276

U2 - 10.1063/5.0268188

DO - 10.1063/5.0268188

M3 - Article

SN - 2378-0967

VL - 10

JO - APL Photonics

JF - APL Photonics

IS - 7

M1 - 070801

ER -

Multi-pass cell driven multi-kHz dispersive wave emission of broadband deep-UV pulses

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