Molecular spectroscopy from 5-12 μm using an OP-GaP OPO

Luke Maidment, Peter G. Schunemann, Derryck Telford Reid

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Abstract

We report a femtosecond optical parametric oscillator (OPO) based on the new semiconductor gain material orientation patterned gallium phosphide (OP-GaP) and being the first example of a broadband OPO operating across the molecular fingerprint region. OP-GaP crystals with lengths of 1 mm and several patterning periods were diced, polished, and anti- reflection (AR) coated for near- to mid-infrared wavelengths. We configured a synchronously pumped OP-GaP OPO in a 101.2-MHz resonator with high reflectivity from 1.15–1.35 μm, pumped with 150-fs pulses from a 1040-nm femtosecond laser (Chromacity Spark). The coating of one spherical mirror was optimized for transmission at the pump wavelength of 1040 nm and for high reflectivity at the resonant signal wavelength in a range from 1.15–1.35 μm, while the other spherical mirror collimated the idler beam emerging from the OP-GaP crystal and was silver coated to provide high reflectivity for all idler wavelengths. This collimated idler beam was output-coupled from the cavity by transmission through a plane mirror coated with high transmission for the idler wavelengths (5–12 μm) and high reflectivity for the signal wavelengths (1.15–1.35 μm) on an infrared-transparent ZnSe substrate. Idler spectra centered from 5.4–11.8 μm and extending to 12.5 μm were collected. The maximum average power was 55 mW at 5.4 μm with 7.5 mW being recorded at 11.8 μm. Details of Fourier transform spectroscopy using water vapor and a polystyrene reference standard are presented.
Original languageEnglish
Title of host publicationNonlinear Frequency Generation and Conversion
Subtitle of host publicationMaterials and Devices XVI
EditorsKonstantin L. Vodopyanov, Kenneth L. Schepler
PublisherSPIE
ISBN (Electronic)9781510606173
DOIs
Publication statusPublished - 20 Feb 2017

Publication series

NameProceedings of SPIE
PublisherSPIE
Volume10088
ISSN (Print)0277-786X
ISSN (Electronic)1996-756X

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    Maidment, L., Schunemann, P. G., & Reid, D. T. (2017). Molecular spectroscopy from 5-12 μm using an OP-GaP OPO. In K. L. Vodopyanov, & K. L. Schepler (Eds.), Nonlinear Frequency Generation and Conversion: Materials and Devices XVI [100880Y] (Proceedings of SPIE; Vol. 10088). SPIE. https://doi.org/10.1117/12.2255892