Abstract
We establish design principles for light-harvesting antennae whose energy capture scales superlinearly with system size. Controlling the absorber dipole orientations produces sets of "guide-slide" states that promote steady-state superabsorbing characteristics in noisy condensed-matter nanostructures. Inspired by natural photosynthetic complexes, we discuss the example of ringlike dipole arrangements and show that, in our setup, vibrational relaxation enhances rather than impedes performance. Remarkably, the superabsorption effect proves to be robust to O(5%) disorder simultaneously for all relevant system parameters, showing promise for experimental exploration across a broad range of platforms.
Original language | English |
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Pages (from-to) | 4323-4329 |
Number of pages | 7 |
Journal | Journal of Physical Chemistry Letters |
Volume | 10 |
Issue number | 15 |
Early online date | 28 Jun 2019 |
DOIs | |
Publication status | Published - 1 Aug 2019 |
ASJC Scopus subject areas
- General Materials Science
- Physical and Theoretical Chemistry
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Datasets for "Light-Harvesting with Guide-Slide Superabsorbing Condensed-Matter Nanostructures"
Gauger, E. (Creator) & Brown, W. (Creator), Heriot-Watt University, 5 Jul 2019
DOI: 10.17861/d90335bb-d3b6-4b0f-883a-c23fac3cba39
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Profiles
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Erik Gauger
- School of Engineering & Physical Sciences - Professor
- School of Engineering & Physical Sciences, Institute of Photonics and Quantum Sciences - Professor
Person: Academic (Research & Teaching)