Giant multiphoton absorption for THz resonances in silicon hydrogenic donors

M. A.W. Van Loon, N. Stavrias, Nguyen H. Le, K. L. Litvinenko, P. T. Greenland, C. R. Pidgeon, K. Saeedi, B. Redlich, G. Aeppli, B. N. Murdin

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Abstract

The absorption of multiple photons when there is no resonant intermediate state is a well-known nonlinear process in atomic vapours, dyes and semiconductors. The N-photon absorption (NPA) rate for donors in semiconductors scales proportionally from hydrogenic atoms in vacuum with the dielectric constant and inversely with the effective mass, factors that carry exponents 6N and 4N, respectively, suggesting that extremely large enhancements are possible. We observed 1PA, 2PA and 3PA in Si:P with a terahertz free-electron laser. The 2PA coefficient for 1s-2s at 4.25 THz was 400,000,000 GM (=4 × 10-42 cm4 s), many orders of magnitude larger than is available in other systems. Such high cross-sections allow us to enter a regime where the NPA cross-section exceeds that of 1PA - that is, when the intensity approaches the binding energy per Bohr radius squared divided by the uncertainty time (only 3.84 MW cm-2 in silicon) - and will enable new kinds of terahertz quantum control.

Original languageEnglish
Pages (from-to)179-184
Number of pages6
JournalNature Photonics
Volume12
Issue number3
Early online date26 Feb 2018
DOIs
Publication statusE-pub ahead of print - 26 Feb 2018

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Atomic and Molecular Physics, and Optics

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    Van Loon, M. A. W., Stavrias, N., Le, N. H., Litvinenko, K. L., Greenland, P. T., Pidgeon, C. R., Saeedi, K., Redlich, B., Aeppli, G., & Murdin, B. N. (2018). Giant multiphoton absorption for THz resonances in silicon hydrogenic donors. Nature Photonics, 12(3), 179-184. https://doi.org/10.1038/s41566-018-0111-x