Enhanced Nonlinear Refractive Index in Epsilon-Near-Zero Materials

  • Lucia Caspani
  • , Muhammad Rishad Kaipurath
  • , Matteo Clerici
  • , Marcello Ferrera
  • , Thomas Roger
  • , J. Kim
  • , Nathaniel Kinsey
  • , Monika Pietrzyk
  • , Andrea Di Falco
  • , Vladimir M. Shalaev
  • , Alexandra Boltasseva
  • , Daniele Franco Angelo Faccio

Research output: Contribution to journalArticlepeer-review

449 Citations (Scopus)
336 Downloads (Pure)

Abstract

New propagation regimes for light arise from the ability to tune the dielectric permittivity toextremely low values. Here we demonstrate a universal approach based on the low linear permittivityvalues attained in the epsilon-near-zero (ENZ) regime for enhancing the nonlinear refractive index,which enables remarkable light-induced changes of the material properties. Experiments performedon Al-doped ZnO (AZO) thin films show a six-fold increase of the Kerr nonlinear refractive index(n2) at the ENZ wavelength, located in the 1300 nm region. This in turn leads to light-inducedrefractive index changes of the order of unity, thus representing a new paradigm for nonlinear optics.
Original languageEnglish
Article number233901
JournalPhysical Review Letters
Volume116
Issue number23
DOIs
Publication statusPublished - 8 Jun 2016

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