TY - JOUR
T1 - A holistic platform for accelerating sorbent-based carbon capture
AU - Charalambous, Charithea
AU - Moubarak, Elias
AU - Schilling, Johannes
AU - Sanchez Fernandez, Eva
AU - Wang, Jin Yu
AU - Herraiz, Laura
AU - Mcilwaine, Fergus
AU - Peh, Shing Bo
AU - Garvin, Matthew
AU - Jablonka, Kevin Maik
AU - Moosavi, Seyed Mohamad
AU - Van Herck, Joren
AU - Ozturk, Aysu Yurdusen
AU - Pourghaderi, Alireza
AU - Song, Ah Young
AU - Mouchaham, Georges
AU - Serre, Christian
AU - Reimer, Jeffrey A.
AU - Bardow, André
AU - Smit, Berend
AU - Garcia, Susana
N1 - Publisher Copyright:
© The Author(s) 2024.
PY - 2024/8/1
Y1 - 2024/8/1
N2 - Reducing carbon dioxide (CO2) emissions urgently requires the large-scale deployment of carbon-capture technologies. These technologies must separate CO2 from various sources and deliver it to different sinks1,2. The quest for optimal solutions for specific source–sink pairs is a complex, multi-objective challenge involving multiple stakeholders and depends on social, economic and regional contexts. Currently, research follows a sequential approach: chemists focus on materials design3 and engineers on optimizing processes4,5, which are then operated at a scale that impacts the economy and the environment. Assessing these impacts, such as the greenhouse gas emissions over the plant’s lifetime, is typically one of the final steps6. Here we introduce the PrISMa (Process-Informed design of tailor-made Sorbent Materials) platform, which integrates materials, process design, techno-economics and life-cycle assessment. We compare more than 60 case studies capturing CO2 from various sources in 5 global regions using different technologies. The platform simultaneously informs various stakeholders about the cost-effectiveness of technologies, process configurations and locations, reveals the molecular characteristics of the top-performing sorbents, and provides insights on environmental impacts, co-benefits and trade-offs. By uniting stakeholders at an early research stage, PrISMa accelerates carbon-capture technology development during this critical period as we aim for a net-zero world.
AB - Reducing carbon dioxide (CO2) emissions urgently requires the large-scale deployment of carbon-capture technologies. These technologies must separate CO2 from various sources and deliver it to different sinks1,2. The quest for optimal solutions for specific source–sink pairs is a complex, multi-objective challenge involving multiple stakeholders and depends on social, economic and regional contexts. Currently, research follows a sequential approach: chemists focus on materials design3 and engineers on optimizing processes4,5, which are then operated at a scale that impacts the economy and the environment. Assessing these impacts, such as the greenhouse gas emissions over the plant’s lifetime, is typically one of the final steps6. Here we introduce the PrISMa (Process-Informed design of tailor-made Sorbent Materials) platform, which integrates materials, process design, techno-economics and life-cycle assessment. We compare more than 60 case studies capturing CO2 from various sources in 5 global regions using different technologies. The platform simultaneously informs various stakeholders about the cost-effectiveness of technologies, process configurations and locations, reveals the molecular characteristics of the top-performing sorbents, and provides insights on environmental impacts, co-benefits and trade-offs. By uniting stakeholders at an early research stage, PrISMa accelerates carbon-capture technology development during this critical period as we aim for a net-zero world.
UR - http://www.scopus.com/inward/record.url?scp=85198852966&partnerID=8YFLogxK
U2 - 10.1038/s41586-024-07683-8
DO - 10.1038/s41586-024-07683-8
M3 - Article
AN - SCOPUS:85198852966
SN - 0028-0836
VL - 632
SP - 89
EP - 94
JO - Nature
JF - Nature
IS - 8023
ER -