A comprehensive study of source apportionment, spatial distribution, and health risks assessment of heavy metal(loid)s in the surface soils of a semi-arid mining region in Matehuala, Mexico

Arnab Saha, Bhaskar Sen Gupta, Sandhya Patidar, Jejanny Lucero Hernández-Martínez, Francisco Martín-Romero, Diana Meza-Figueroa, Nadia Martínez-Villegas

Research output: Contribution to journalArticlepeer-review

2 Citations (Scopus)

Abstract

Background
This study investigates the contamination level, spatial distribution, pollution sources, potential ecological risks, and human health risks associated with heavy metal(loid)s (i.e., arsenic (As), copper (Cu), iron (Fe), manganese (Mn), lead (Pb), and zinc (Zn)) in surface soils within the mining region of Matehuala, located in central Mexico.

Objectives
The primary objectives are to estimate the contamination level of heavy metal(loid)s, identify pollution sources, assess potential ecological risks, and evaluate human health risks associated with heavy metal(loid) contamination.

Methods
Soil samples from the study area were analysed using various indices including Igeo, Cf, PLI, mCd, EF, and PERI to evaluate contamination levels. Source apportionment of heavy metal(loid)s was conducted using the APCS-MLR and PMF receptor models. Spatial distribution patterns were determined using the most efficient interpolation technique among five different approaches. The total carcinogenic risk index (TCR) and total non-carcinogenic index (THI) were used in this study to assess the potential carcinogenic and non-carcinogenic hazards posed by heavy metal(loid)s in surface soil to human health.

Results
The study reveals a high contamination level of heavy metal(loid)s in the surface soil, posing considerable ecological risks. As was identified as a priority metal for regulatory control measures. Mining and smelting activities were identified as the primary factors influencing heavy metal(loid) distributions. Based on spatial distribution mapping, concentrations were higher in the northern, western, and central regions of the study area. As and Fe were found to pose considerable and moderate ecological risks, respectively. Health risk evaluation indicated significant levels of carcinogenic risks for both adults and children, with higher risks for children.

Conclusion
This study highlights the urgent need for monitoring heavy metal(loid) contamination in Matehuala's soils, particularly in regions experiencing strong economic growth, to mitigate potential human health and ecological risks associated with heavy metal(loid) pollution.
Original languageEnglish
Article number119619
JournalEnvironmental Research
Volume260
Early online date14 Jul 2024
DOIs
Publication statusE-pub ahead of print - 14 Jul 2024

Keywords

  • Heavy metal(loid)s
  • Source apportionment
  • Spatial distribution
  • Risk assessment
  • Mining region

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